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Document Details
Document Type
:
Article In Journal
Document Title
:
Attachment to manganese or cobalt of a bulky tri(organosilyl)methyl ligand containing an NMe2 or an OMe donor group
Attachment to manganese or cobalt of a bulky tri(organosilyl)methyl ligand containing an NMe2 or an OMe donor group
Document Language
:
Arabic
Abstract
:
The organolithium compound Li(THF)(2){C(SiMe3)(2)(SiMe2NMe2)} reacted with one equivalent of MnCl2 to give [Mn(mu-Cl){C(SiMe3)(2)(SiMe2NMe2)}](2) (4) and with 0.5 equivalent of MnCl2 to give Mn{C(SiMe3)(2)(SiMe2NMe2)}(2) together with a small amount of the Mn-III compound [Mn(mu-O){C(SiMe3)(2)(SiMe2NMe2)}](2) (6) formed by adventitious admission of air. With CoBr2, the compound [Co(mu-Br){C(SiMe3)(2)(SiMe2NMe2)}](2) (7) was obtained. The reaction between the lithium compound Li(THF)(2){C(SiMe3)(2)(SiMe2OMe)} and MnCl2 in THF gave [Mn(THF)(mu-Cl){C(SiMe3)(2)(SiMe2OMe)}](2) (5). The crystal structures of compounds 4, 5, 6 and 7 were determined. Compounds 4 and 5 are the first manganese analogues of Grignard reagents containing Mn-C sigma-bonds to be characterised in the solid state. (C) 2002 Elsevier Science B.V. All rights reserved.
Journal Name
:
JOURNAL OF ORGANOMETALLIC CHEMISTRY
Volume
:
649
Issue Number
:
2
Publishing Year
:
2002 AH
Added Date
:
Saturday, June 14, 2008
Researchers
Researcher Name (Arabic)
Researcher Name (English)
Researcher Type
Dr Grade
Email
صالح بن سـالــم نـافـل الجعيـــد
Al-Juaid SS
Researcher
saljuaid@kau.edu.sa
.
Eaborn C
Researcher
.
El-Hamruni SM
Researcher
.
Hitchcock PB
Researcher
.
Smith JD
Researcher
.
Can SES
Researcher
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